For spine chilling, still have to say I’ll go with Gregorian Chant.
Definitely. There’s an Enya song very similar in sound to Gregorian chant that’s notorious for being used as a backdrop to a lot of raps actually.
This an instrumental sample:
https://youtube.com/shorts/jqlYVYwi4jg?si=do_7p9jY3tOJVDmK