Sure you could. He ran for President under fraudulant circumstances. Fraud is certainly a "High Crime or Misdemeanor".
I've read the USC a few times in my life. The only provision for removing a sitting president is impeachment in the House, conviction in the Senate.
Actually, there is nothing in the Constitution that would prohibit a sitting President from being arrested, by any law enforcement officer.
The problem is, the President could then issue himself a prompt “pardon” and things would get messy.
Better to have the cabinet act, if it needed to be done quickly.