That's not what the word means. "Incredulous" here is a description of the reaction of the viewer, not of Brit's speaking manner. Words that would work include "incredibly", "unbelievably", and quite a few others.
I think it's being used to describe Brit's reaction.
I didn't see the show, but from the description ('Kristol questioned ... smear tactic'), I would assume that Kristol made some comment or accusation to that effect, and Hume was incredulous (disbelieving, expression of disbelief) that BK would infer he was involved in a smear campaign.
IMHO, of course.