My personal favs (in no order) are Sinatra - You Only Live Twice, Simon - Nobody Does it Better, Bassey - Diamonds Are Forever, Easton - For Your Eyes Only and Coolidge - All Time High. Surprisingly I kinda like that one Garbage did...ummm... World is Not Enough.
Adele and Skyfall is way up there. Better than the movie until I watch it. When is it out on BluRay?, LOL!
Live and Let Die, nothing else comes close.
My favorite is “You Only Live Twice”
Here is a vid of the opening sequence in HD
http://www.youtube.com/watch?v=6aufH98vkyg
I’ve spun Bassey’s “Goldfinger” on the turntable many times.
http://www.youtube.com/watch?v=Fy_PJODH3p0